Cloning and characterization of an n-alkane-inducible cytochrome P450 gene essential for n-decane assimilation by Yarrowia lipolytica

Yeast. 1998 Nov;14(15):1387-97. doi: 10.1002/(SICI)1097-0061(199811)14:15<1387::AID-YEA333>3.0.CO;2-M.

Abstract

A gene encoding cytochrome P450 involved in n-alkane utilization was cloned from an n-alkane assimilating yeast, Yarrowia lipolytica CX161-1B. The RT-PCR was performed on the mRNA prepared from the cells grown on n-alkane as a template using degenerated PCR primers designed for the conserved amino acid sequences of the CYP52 family. The RT-PCR amplified fragment was then used as a probe to isolate genes coding for P450 of the CYP52 family from the genomic DNA library of the strain CX161-1B. The nucleotide sequence of one of the positive clones was determined. An open reading frame which had the same nucleotide sequence as the RT-PCR-amplified fragment was identified. It was of 523 amino acid residues, 60.2 kDa in molecular mass, and had 30-45% sequence identity with the other members of the CYP52 family of Candida species so far analysed. The expression of the P450 gene that was named as YlALK1 was induced by n-tetradecane and repressed by glycerol. A YlALK1 gene disruptant did not grow well on n-decane, but grew on longer-chain n-alkanes such as hexadecane as a sole carbon source. Introduction of YlALK1 on a plasmid to the disruptant restored the decane assimilation. These results suggest that the YlALK1 gene product is the major P450A1k to metabolize short-chain n-alkanes such as decane and dodecane in Y. lipolytica.

MeSH terms

  • Alkanes / metabolism*
  • Amino Acid Sequence
  • Base Sequence
  • Cloning, Molecular
  • Cytochrome P-450 Enzyme System / genetics*
  • Cytochrome P-450 Enzyme System / metabolism
  • Electroporation
  • Enzyme Induction
  • Gene Deletion
  • Genes, Fungal
  • Molecular Sequence Data
  • RNA, Messenger / isolation & purification
  • RNA, Messenger / metabolism
  • Restriction Mapping
  • Reverse Transcriptase Polymerase Chain Reaction / methods
  • Saccharomycetales / enzymology
  • Saccharomycetales / genetics*
  • Saccharomycetales / growth & development
  • Sequence Alignment

Substances

  • Alkanes
  • RNA, Messenger
  • n-tetradecane
  • Cytochrome P-450 Enzyme System
  • decane

Associated data

  • GENBANK/AB010388