Que L Jr - Search Results

1

10-Fold Increase in Hydrogen Atom Transfer Reactivity for a Series of S = 1 Fe^IV═O Complexes Over the S = 2 [(TQA)Fe^IV═O]²⁺ Complex via Entropic Lowering of Reaction Barriers by Secondary Sphere Cycloalkyl Substitution.

Das A, Pal N, Xiong J, Young VG Jr, Guo Y, Swart M, Que L Jr. Das A, et al. Among authors: que l jr. J Am Chem Soc. 2024 Dec 19. doi: 10.1021/jacs.4c10120. Online ahead of print. J Am Chem Soc. 2024. PMID: 39699233

2

Experimental Definition of the S = 1 π vs S = 2 σ Reactivity and S = 2 Character in the Ground State of an S = 1 Fe^IVO Complex.

Braun A, Gee LB, Waters MDJ, Baker ML, Mara MW, Zhou A, Kroll T, Nordlund D, Sokaras D, Hedman B, Hodgson KO, Que L Jr, Solomon EI. Braun A, et al. Among authors: que l jr. J Am Chem Soc. 2024 Dec 13. doi: 10.1021/jacs.4c11034. Online ahead of print. J Am Chem Soc. 2024. PMID: 39668699

3

Preparation and characterization of Mn^IIMn^III complexes with relevance to class Ib ribonucleotide reductases.

Doyle LM, Bienenmann RLM, Gericke R, Xu S, Farquhar ER, Que L Jr, McDonald AR. Doyle LM, et al. Among authors: que l jr. J Inorg Biochem. 2024 Aug;257:112583. doi: 10.1016/j.jinorgbio.2024.112583. Epub 2024 May 5. J Inorg Biochem. 2024. PMID: 38733704 Free article.

4

A tale of two topological isomers: Uptuning [Fe^IV(O)(Me₄cyclam)]²⁺ for olefin epoxidation.

Chandra B, Ahsan F, Sheng Y, Swart M, Que L Jr. Chandra B, et al. Among authors: que l jr. Proc Natl Acad Sci U S A. 2024 Mar 19;121(12):e2319799121. doi: 10.1073/pnas.2319799121. Epub 2024 Mar 13. Proc Natl Acad Sci U S A. 2024. PMID: 38478690 Free PMC article.

5

NMR and Mössbauer Studies Reveal a Temperature-Dependent Switch from S = 1 to 2 in a Nonheme Oxoiron(IV) Complex with Faster C-H Bond Cleavage Rates.

Rasheed W, Pal N, Aboelenen AM, Banerjee S, Oloo WN, Klein JEMN, Fan R, Xiong J, Guo Y, Que L Jr. Rasheed W, et al. Among authors: que l jr. J Am Chem Soc. 2024 Feb 14;146(6):3796-3804. doi: 10.1021/jacs.3c10694. Epub 2024 Feb 1. J Am Chem Soc. 2024. PMID: 38299607 Free PMC article.

6

Class Ib Ribonucleotide Reductases: Activation of a Peroxido-Mn^IIMn^III to Generate a Reactive Oxo-Mn^IIIMn^IV Oxidant.

Doyle L, Magherusan A, Xu S, Murphy K, Farquhar ER, Molton F, Duboc C, Que L Jr, McDonald AR. Doyle L, et al. Among authors: que l jr. Inorg Chem. 2024 Jan 29;63(4):2194-2203. doi: 10.1021/acs.inorgchem.3c04163. Epub 2024 Jan 17. Inorg Chem. 2024. PMID: 38231137 Free PMC article.

7

10⁶-fold faster C-H bond hydroxylation by a Co^III,IV₂(µ-O)₂ complex [via a Co^III₂(µ-O)(µ-OH) intermediate] versus its Fe^IIIFe^IV analog.

Li Y, Abelson C, Que L Jr, Wang D. Li Y, et al. Among authors: que l jr. Proc Natl Acad Sci U S A. 2023 Dec 19;120(51):e2307950120. doi: 10.1073/pnas.2307950120. Epub 2023 Dec 12. Proc Natl Acad Sci U S A. 2023. PMID: 38085777 Free PMC article.

8

Formation of a Reactive [Mn(III)-O-Ce(IV)] Species and its Facile Equilibrium with Related Mn(IV)(OX) (X = Sc or H) Complexes.

Gupta S, Arora P, Kumar R, Awasthi A, Chandra B, Eerlapally R, Xiong J, Guo Y, Que L Jr, Draksharapu A. Gupta S, et al. Among authors: que l jr. Angew Chem Int Ed Engl. 2024 Jan 15;63(3):e202316378. doi: 10.1002/anie.202316378. Epub 2023 Dec 7. Angew Chem Int Ed Engl. 2024. PMID: 37997195

9

Explorations of the nonheme high-valent iron-oxo landscape: crystal structure of a synthetic complex with an [FeIV2(μ-O)₂] diamond core relevant to the chemistry of sMMOH.

Rohde GT, Xue G, Que L Jr. Rohde GT, et al. Among authors: que l jr. Faraday Discuss. 2022 May 18;234(0):109-128. doi: 10.1039/d1fd00066g. Faraday Discuss. 2022. PMID: 35171169 Free PMC article.

10

Nonheme Diiron Oxygenase Mimic That Generates a Diferric-Peroxo Intermediate Capable of Catalytic Olefin Epoxidation and Alkane Hydroxylation Including Cyclohexane.

Oloo WN, Szávuly M, Kaizer J, Que L Jr. Oloo WN, et al. Among authors: que l jr. Inorg Chem. 2022 Jan 10;61(1):37-41. doi: 10.1021/acs.inorgchem.1c03468. Epub 2021 Dec 11. Inorg Chem. 2022. PMID: 34894683 Free PMC article.

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